The only causes that can potentially kill shrimps are high CO2, low O2, NH3/NH4 and NO2. Since you did multiple large water changes, the excel effect should have gone off. The only possible explanation is that your bacteria count drop substantially and that small spikes in NH3/NH4 did them in. (The other possible thing is low O2...do you have some good surface movement?). All in all, you have poor plant growth to start with. If you use CO2 gas, learn to use it well.
Regards
Peter Gwee
Plant Physiology by Taiz and Zeiger
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